Optimization of Sb2Te3 and Bi2Te3 thermoelectric films for infrared detection and energy harvesting
摘要
We are developing antenna-coupled thermoelectric junctions for infrared detection and energy harvesting. Joule heating at the antenna feed from currents induced by antenna-collected radiation generates thermoelectric voltage and current for detection and energy conversion. COMSOL Multiphysics simulations identify Sb2Te3 and Bi2Te3 thermoelectric materials as ideal for the thermocouple junction at the antenna feed. We optimized RF sputtered telluride films by performing a 2-level full-factorial experiment with three factors–argon pressure, substrate temperature, and RF power—with power factor as the response. Preliminary photolithographically patterned devices designed for mm-waves using less suitable materials gave immeasurably low response to radiation from a backward wave oscillator, which is explained by the simulations that motivate this study.
Graphical abstractWe are developing antenna-coupled thermoelectric junctions for infrared detection and energy harvesting. Joule heating at the antenna feed from currents induced by antenna-collected radiation generates thermoelectric voltage and current for detection and energy conversion. COMSOL Multiphysics simulations identify Sb2Te3 and Bi2Te3 thermoelectric materials as ideal for the thermocouple junction at the antenna feed. We optimized RF sputtered telluride films by performing a 2-level full-factorial experiment with three factors—argon pressure, substrate temperature, and RF power—with power factor as the response. Preliminary photolithographically patterned devices designed for mm-waves using less suitable materials gave immeasurably low response to radiation from a backward wave oscillator, which is explained by the simulations that motivate this study.