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<p>Photon avalanche (PA) upconversion, driven by a positive feedback loop that couples nonresonant ground-state absorption (GSA), resonant excited-state absorption (ESA), and highly efficient cross-relaxation (CR), gives rise to a threshold-triggered ultrahigh optical nonlinearity accompanied by uniquely prolonged rise-time dynamics. From spark to surge, this phenomenon can deliver tens to even hundreds of nonlinear orders at the nanoscale, redefining opportunities in imaging, sensing, and optical computing while opening a new paradigm for interrogating light–matter interactions.</p>

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Photon avalanche nanomaterials: from spark to surge

  • 期刊论文

  • 出版模式：

    开放获取

  • 发表日期：

    2025年11月10日

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  • Chang Liu,
  • Yuzheng Wang,
  • Yixun Fan,
  • Liangliang Liang

摘要

Photon avalanche (PA) upconversion, driven by a positive feedback loop that couples nonresonant ground-state absorption (GSA), resonant excited-state absorption (ESA), and highly efficient cross-relaxation (CR), gives rise to a threshold-triggered ultrahigh optical nonlinearity accompanied by uniquely prolonged rise-time dynamics. From spark to surge, this phenomenon can deliver tens to even hundreds of nonlinear orders at the nanoscale, redefining opportunities in imaging, sensing, and optical computing while opening a new paradigm for interrogating light–matter interactions.