Abstract <p> Experimental studies of magnetic properties of a topological van der Waals antiferromagnet insulator MnBi<InlineEquation ID="IEq3"> <EquationSource Format="TEX">\(_2\)</EquationSource> </InlineEquation>Te<InlineEquation ID="IEq4"> <EquationSource Format="TEX">\(_4\)</EquationSource> </InlineEquation> demonstrated not only an anomalous behavior of magnetization before and after the spin-flop transition but also its strong temperature dependence. To interpret these effects, we present a quantum theory of layered antiferromagnet with a trigonal symmetry of the triangular lattice. Using atomic representations for spin operators and the diagram technique for Hubbard operators, we obtain a dispersion equation describing the temperature dependence of the excitation spectrum. In the anisotropic self-consistent field approximation, we derive a transcendent equation establishing an interrelation between the Néel temperature and model parameters. For the weak-anisotropy case, we obtain its analytical solution. We describe the temperature evolution of magnetization as a function of magnetic field and construct a phase diagram showing regions where different configurations of MnBi<InlineEquation ID="IEq5"> <EquationSource Format="TEX">\(_2\)</EquationSource> </InlineEquation>Te<InlineEquation ID="IEq6"> <EquationSource Format="TEX">\(_4\)</EquationSource> </InlineEquation> magnetic sublattices are realized. We observe that quantum effects induced by the trigonal component of the single-ion anisotropy essentially affect the thermodynamic properties of antiferromagnets. </p>

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Temperature dependence of the spin-flop transition in a topological antiferromagnet MnBi\(_2\)Te\(_4\)

  • V. V. Val’kov,
  • A. O. Zlotnikov,
  • A. Gamov

摘要

Abstract

Experimental studies of magnetic properties of a topological van der Waals antiferromagnet insulator MnBi \(_2\) Te \(_4\) demonstrated not only an anomalous behavior of magnetization before and after the spin-flop transition but also its strong temperature dependence. To interpret these effects, we present a quantum theory of layered antiferromagnet with a trigonal symmetry of the triangular lattice. Using atomic representations for spin operators and the diagram technique for Hubbard operators, we obtain a dispersion equation describing the temperature dependence of the excitation spectrum. In the anisotropic self-consistent field approximation, we derive a transcendent equation establishing an interrelation between the Néel temperature and model parameters. For the weak-anisotropy case, we obtain its analytical solution. We describe the temperature evolution of magnetization as a function of magnetic field and construct a phase diagram showing regions where different configurations of MnBi \(_2\) Te \(_4\) magnetic sublattices are realized. We observe that quantum effects induced by the trigonal component of the single-ion anisotropy essentially affect the thermodynamic properties of antiferromagnets.