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Sulfonium Derivatives of the closo-Decaborate Anion with Carbonyl Groups

  • A. S. Kubasov,
  • A. V. Golubev,
  • O. M. Stepanova,
  • K. Yu. Zhizhin,
  • N. T. Kuznetsov

摘要

Abstract

This paper presents the synthesis of sulfonium derivatives of the closo-decaborate anion with exo-polyhedral carbonyl groups [B10H9S(CH2C(=O)R)2] (R = Me, Ph, p-C6H4Cl, Nh). The composition and structure have been confirmed by elemental analysis, 11B, 1H, and 13C NMR spectroscopies. Crystal packings and intermolecular interactions for compounds Bu4N[2-B10H9S(CH2COMe)2] and [Ag(PPh3)4][2-B10H9S(CH2COC6H4Cl)2] have been studied using single crystal X-ray diffraction and Hirschfeld surface analysis of the anions.