Coral records indicate six-decade rise and fall of atmospheric lead emission in China
摘要
Despite the global ban on leaded gasoline, environmental lead pollution remains a concern, especially in developing countries. Asia, and particularly China, has emerged as a major emission center, yet long-term records of atmospheric lead emission are scarce and often inconsistent. Here we reconstruct a 60-year history of lead concentration (lead/calcium) and isotopic composition in a coral from Dongsha Atoll in the northern South China Sea. The record shows a fourfold increase in lead level from 1953 to the mid-2000s, followed by a ~60% decline over the next decade. Shifts in lead isotopic composition suggest a transition from local automotive emissions to more distant industrial emissions, primarily from coal combustion in mainland China after 2000. This industrial source has declined significantly after the mid-2000s in response to stricter air pollution controls. Our findings highlight both the lasting legacy of leaded gasoline and the effectiveness of recent environmental policies in reducing atmospheric lead exposure.