<p>The quasi-one-dimensional charge density wave (CDW) material (TaSe<sub>4</sub>)<sub>2</sub>I has been recently predicted to host Kramers-Weyl (KW) fermions which should exist in the vicinity of high symmetry points in the Brillouin zone in chiral materials with strong spin-orbit coupling. However, direct spectroscopic evidence of KW fermions is limited. Here we use helicity-dependent laser-based angle-resolved photoemission spectroscopy (ARPES) in conjunction with tight-binding and first-principles calculations to identify KW fermions in (TaSe<sub>4</sub>)<sub>2</sub>I. We find that topological and symmetry considerations place distinct constraints on the (pseudo-) spin texture and the observed spectra around a KW node. Our findings highlight the unique topological nature of (TaSe<sub>4</sub>)<sub>2</sub>I and provide a pathway for identifying KW fermions in other chiral materials.</p>

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Signatures of Kramers-Weyl fermions in the charge density wave material (TaSe4)2I

  • Soyeun Kim,
  • Robert C. McKay,
  • Nina Bielinski,
  • Junehu Park,
  • Chengxi Zhao,
  • Meng-Kai Lin,
  • Joseph A. Hlevyack,
  • Xuefei Guo,
  • Sung-Kwan Mo,
  • Peter Abbamonte,
  • T.-C. Chiang,
  • André Schleife,
  • Daniel P. Shoemaker,
  • Barry Bradlyn,
  • Fahad Mahmood

摘要

The quasi-one-dimensional charge density wave (CDW) material (TaSe4)2I has been recently predicted to host Kramers-Weyl (KW) fermions which should exist in the vicinity of high symmetry points in the Brillouin zone in chiral materials with strong spin-orbit coupling. However, direct spectroscopic evidence of KW fermions is limited. Here we use helicity-dependent laser-based angle-resolved photoemission spectroscopy (ARPES) in conjunction with tight-binding and first-principles calculations to identify KW fermions in (TaSe4)2I. We find that topological and symmetry considerations place distinct constraints on the (pseudo-) spin texture and the observed spectra around a KW node. Our findings highlight the unique topological nature of (TaSe4)2I and provide a pathway for identifying KW fermions in other chiral materials.