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Intrinsically stretchable quantum dot light-emitting diodes

  • Dong Chan Kim,
  • Hyojin Seung,
  • Jisu Yoo,
  • Junhee Kim,
  • Hyeon Hwa Song,
  • Ji Su Kim,
  • Yunho Kim,
  • Kyunghoon Lee,
  • Changsoon Choi,
  • Dongjun Jung,
  • Chansul Park,
  • Hyeonjun Heo,
  • Jiwoong Yang,
  • Taeghwan Hyeon,
  • Moon Kee Choi,
  • Dae-Hyeong Kim

摘要

Stretchable displays that can change their shape and size under strain could be used to create displays with unconventional form factors. However, intrinsically stretchable light-emitting devices have poor luminous performance, such as low brightness. Here we show that intrinsically stretchable quantum dot light-emitting diodes (QLEDs) can be made using a mechanically soft and stretchable emissive layer consisting of a ternary nanocomposite of colloidal quantum dots, an elastomeric polymer and a charge transport polymer. The light-emitting layer maintains a nearly constant interparticle distance even under 50% strain, ensuring reliable operation of the QLED under stretching. The polymer-rich charge transport region at the bottom of the nanocomposite functions as a hole transport pathway to the embedded quantum dots. The QLEDs exhibit a turn-on voltage of 3.2 V and a maximum luminance of 15,170 cd m−2 at 6.2 V without loss of brightness, even when under 50% strain, and can be used to make stretchable full-colour passive-matrix QLED arrays.