<p>Glutaric aciduria type 1 is caused by inherited deficiency of glutaryl-CoA dehydrogenase and subsequent accumulation of neurotoxic metabolites. Clinically, the disease is characterized by striatal damage and dystonic movement disorder in untreated infants. Despite newborn screening and pre-symptomatic therapy start, about one-third of patients still develop neurological symptoms. Furthermore, progressive white matter changes and chronic kidney disease highlights the need for improved therapies. To elucidate the potential of substrate reduction therapy for GA1 we investigated whether aminoadipate-semialdehyde synthetase, the first enzyme of the lysine oxidation pathway, could serve as therapeutic target. Therefore, we studied whether <i>Gcdh</i> knockout (KO) mice, a known animal model for GA1, were rescued by additional knockout of <i>Aass</i>. <i>Gcdh/Aass</i> KO mice were clinically indistinguishable from wild-type mice and showed a marked reduction of glutaric acid in brain (20.9&#xa0;µg/mg protein vs. 59.2&#xa0;µg/mg protein; <i>p</i> = 0.001), liver (23.5&#xa0;µg/mg protein vs. 104.8&#xa0;µg/mg protein; <i>p</i> = 0.001), and urine (11.9&#xa0;mol/mol creatinine vs. 166.5&#xa0;mol/mol creatinine; <i>p</i> = 0.001). The effect was less pronounced for 3-hydroxyglutaric acid. Unlike <i>Gcdh</i> KO mice, <i>Gcdh/Aass</i> KO mice did not develop a severe phenotype under high-lysine diet. In conclusion, knockout of <i>Aass</i> partially rescues the severe phenotype of <i>Gcdh</i> KO mice, providing a potential therapeutic target.</p>

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Aminoadipate-semialdehyde synthase, a potential target for substrate reduction therapy in glutaric aciduria type 1

  • Celine Saad,
  • Sabine Jung-Klawitter,
  • Bianca Dimitrov,
  • Juan Antonio Aguilar-Pimentel,
  • Lore Becker,
  • Patricia da Silva-Buttkus,
  • Nathalia R. V. Dragano,
  • Lillian Garrett,
  • Sabine M. Hölter,
  • Birgit Rathkolb,
  • Adrián Sanz-Moreno,
  • Nadine Spielmann,
  • Helmut Fuchs,
  • Valerie Gailus-Durner,
  • Christian P. Schaaf,
  • Giancarlo la Marca,
  • Roberta Damiano,
  • Dirk J. Lefeber,
  • Udo Engelke,
  • Clara C. D. M. van Karnebeek,
  • Alex Garanto Iglesias,
  • Carole Linster,
  • Curtis R. Coughlin II,
  • Blair R. Leavitt,
  • Christina Fillat,
  • Martin Hrabe de Angelis,
  • Sander M. Houten,
  • Stefan Kölker

摘要

Glutaric aciduria type 1 is caused by inherited deficiency of glutaryl-CoA dehydrogenase and subsequent accumulation of neurotoxic metabolites. Clinically, the disease is characterized by striatal damage and dystonic movement disorder in untreated infants. Despite newborn screening and pre-symptomatic therapy start, about one-third of patients still develop neurological symptoms. Furthermore, progressive white matter changes and chronic kidney disease highlights the need for improved therapies. To elucidate the potential of substrate reduction therapy for GA1 we investigated whether aminoadipate-semialdehyde synthetase, the first enzyme of the lysine oxidation pathway, could serve as therapeutic target. Therefore, we studied whether Gcdh knockout (KO) mice, a known animal model for GA1, were rescued by additional knockout of Aass. Gcdh/Aass KO mice were clinically indistinguishable from wild-type mice and showed a marked reduction of glutaric acid in brain (20.9 µg/mg protein vs. 59.2 µg/mg protein; p = 0.001), liver (23.5 µg/mg protein vs. 104.8 µg/mg protein; p = 0.001), and urine (11.9 mol/mol creatinine vs. 166.5 mol/mol creatinine; p = 0.001). The effect was less pronounced for 3-hydroxyglutaric acid. Unlike Gcdh KO mice, Gcdh/Aass KO mice did not develop a severe phenotype under high-lysine diet. In conclusion, knockout of Aass partially rescues the severe phenotype of Gcdh KO mice, providing a potential therapeutic target.