<p>Incommensurate magnetic phases in chiral cubic crystals are an established source of topological spin textures such as skyrmion and hedgehog lattices, with potential applications in spintronics and information storage. We report a comprehensive small-angle neutron scattering (SANS) study on the <i>B</i>20-type chiral magnet Cr<InlineEquation ID="IEq5"> <InlineMediaObject> <ImageObject Color="BlackWhite" FileRef="41598_2025_86652_Article_IEq5.gif" Format="GIF" Height="10" Rendition="HTML" Resolution="72" Type="Linedraw" Width="23" /> </InlineMediaObject> <EquationSource Format="TEX">\(_{0.82}\)</EquationSource> </InlineEquation>Mn<InlineEquation ID="IEq6"> <InlineMediaObject> <ImageObject Color="BlackWhite" FileRef="41598_2025_86652_Article_IEq6.gif" Format="GIF" Height="10" Rendition="HTML" Resolution="72" Type="Linedraw" Width="23" /> </InlineMediaObject> <EquationSource Format="TEX">\(_{0.18}\)</EquationSource> </InlineEquation>Ge, exploring its magnetic phase diagram and confirming the stabilization of a skyrmion lattice under low magnetic fields. Our results reveal a helical ground state with a decreasing pitch from 40 to 35&#xa0;nm upon cooling, and a skyrmion phase stable in applied magnetic fields of 10–30&#xa0;mT, and over an unusually wide temperature range for chiral magnets of 6 K (<InlineEquation ID="IEq7"> <InlineMediaObject> <ImageObject Color="BlackWhite" FileRef="41598_2025_86652_Article_IEq7.gif" Format="GIF" Height="19" Rendition="HTML" Resolution="72" Type="Linedraw" Width="131" /> </InlineMediaObject> <EquationSource Format="TEX">\(\sim T_\text {C}/2&lt; T &lt; T_\text {C}\)</EquationSource> </InlineEquation>, <InlineEquation ID="IEq8"> <InlineMediaObject> <ImageObject Color="BlackWhite" FileRef="41598_2025_86652_Article_IEq8.gif" Format="GIF" Height="16" Rendition="HTML" Resolution="72" Type="Linedraw" Width="58" /> </InlineMediaObject> <EquationSource Format="TEX">\(T_\text {C}=13\)</EquationSource> </InlineEquation> K). The skyrmion lattice forms a standard two-dimensional hexagonal coordination that can be trained into a single domain, distinguishing it from the three-dimensional hedgehog lattice observed in MnGe-based systems. Additionally, we demonstrate the persistence of a metastable SkL at 2&#xa0;K, even at zero field. These findings advance our understanding of magnetic textures in Cr-based <i>B</i>20 compounds, highlighting Cr<sub>0.82</sub>Mn<sub>0.18</sub>Ge as a promising material for further exploration in topological magnetism.</p>

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Observation of magnetic skyrmion lattice in Cr0.82Mn0.18Ge by small-angle neutron scattering

  • Victor Ukleev,
  • Tapas Samanta,
  • Oleg I. Utesov,
  • Jonathan S. White,
  • Luana Caron

摘要

Incommensurate magnetic phases in chiral cubic crystals are an established source of topological spin textures such as skyrmion and hedgehog lattices, with potential applications in spintronics and information storage. We report a comprehensive small-angle neutron scattering (SANS) study on the B20-type chiral magnet Cr \(_{0.82}\) Mn \(_{0.18}\) Ge, exploring its magnetic phase diagram and confirming the stabilization of a skyrmion lattice under low magnetic fields. Our results reveal a helical ground state with a decreasing pitch from 40 to 35 nm upon cooling, and a skyrmion phase stable in applied magnetic fields of 10–30 mT, and over an unusually wide temperature range for chiral magnets of 6 K ( \(\sim T_\text {C}/2< T < T_\text {C}\) , \(T_\text {C}=13\) K). The skyrmion lattice forms a standard two-dimensional hexagonal coordination that can be trained into a single domain, distinguishing it from the three-dimensional hedgehog lattice observed in MnGe-based systems. Additionally, we demonstrate the persistence of a metastable SkL at 2 K, even at zero field. These findings advance our understanding of magnetic textures in Cr-based B20 compounds, highlighting Cr0.82Mn0.18Ge as a promising material for further exploration in topological magnetism.