<p>Understanding the nature of collective charge dynamics in the Coulomb gap phase is essential for revealing the existence of many-body localization. However, the corresponding many-particle excitation spectra remain poorly understood. Here, we present a comprehensive investigation of <InlineEquation ID="IEq1"> <EquationSource Format="TEX">\(^{27}\)</EquationSource> </InlineEquation>Al and <InlineEquation ID="IEq2"> <EquationSource Format="TEX">\(^{63}\)</EquationSource> </InlineEquation>Cu nuclear magnetic/quadrupole resonance (NMR/NQR), along with specific heat (<InlineEquation ID="IEq3"> <EquationSource Format="TEX">\(C_p\)</EquationSource> </InlineEquation>) measurements, in the <i>p</i>-type semiconductor CuAlO<InlineEquation ID="IEq4"> <EquationSource Format="TEX">\(_2\)</EquationSource> </InlineEquation>. Our study unveils distinct changes in charge dynamics at two crossover temperature scales which separate three regimes associated with Anderson localization of charge carriers: thermally activated transport (<InlineEquation ID="IEq5"> <EquationSource Format="TEX">\(T&gt;150\)</EquationSource> </InlineEquation> K) <InlineEquation ID="IEq6"> <EquationSource Format="TEX">\(\rightarrow\)</EquationSource> </InlineEquation> Mott variable-range hopping (VRH) <InlineEquation ID="IEq7"> <EquationSource Format="TEX">\(\rightarrow\)</EquationSource> </InlineEquation> Efros–Shklovskii (ES) VRH with Coulomb gap formation (<InlineEquation ID="IEq8"> <EquationSource Format="TEX">\(T&lt;50\)</EquationSource> </InlineEquation> K). In the ES VRH regime, we observe a striking divergence in the zero-field <InlineEquation ID="IEq9"> <EquationSource Format="TEX">\(^{63}\)</EquationSource> </InlineEquation>Cu spin-lattice relaxation rate, <InlineEquation ID="IEq10"> <EquationSource Format="TEX">\((T_1T)^{-1}\)</EquationSource> </InlineEquation>, which is strongly suppressed by an applied magnetic field, indicative of quantum critical charge fluctuations. This is further supported by a distinct magnetic field-dependence of <InlineEquation ID="IEq11"> <EquationSource Format="TEX">\(C_p/T\)</EquationSource> </InlineEquation> deep within the Coulomb gap phase. Taken together, these results provide compelling evidence for the emergence of strong, gapless collective charge fluctuations within the Anderson insulating phase where single-particle excitations are gapped.</p>

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Observation of gapless collective charge fluctuations in an Anderson insulating state

  • Jong Mok Ok,
  • Beom Jun Park,
  • Junik Hwang,
  • Seonghoon Park,
  • Myeongjun Kang,
  • Jun Sung Kim,
  • Ki-Seok Kim,
  • Seung-Ho Baek

摘要

Understanding the nature of collective charge dynamics in the Coulomb gap phase is essential for revealing the existence of many-body localization. However, the corresponding many-particle excitation spectra remain poorly understood. Here, we present a comprehensive investigation of \(^{27}\) Al and \(^{63}\) Cu nuclear magnetic/quadrupole resonance (NMR/NQR), along with specific heat ( \(C_p\) ) measurements, in the p-type semiconductor CuAlO \(_2\) . Our study unveils distinct changes in charge dynamics at two crossover temperature scales which separate three regimes associated with Anderson localization of charge carriers: thermally activated transport ( \(T>150\) K) \(\rightarrow\) Mott variable-range hopping (VRH) \(\rightarrow\) Efros–Shklovskii (ES) VRH with Coulomb gap formation ( \(T<50\) K). In the ES VRH regime, we observe a striking divergence in the zero-field \(^{63}\) Cu spin-lattice relaxation rate, \((T_1T)^{-1}\) , which is strongly suppressed by an applied magnetic field, indicative of quantum critical charge fluctuations. This is further supported by a distinct magnetic field-dependence of \(C_p/T\) deep within the Coulomb gap phase. Taken together, these results provide compelling evidence for the emergence of strong, gapless collective charge fluctuations within the Anderson insulating phase where single-particle excitations are gapped.