<p>Optical control offers a non-contact, high-precision and ultrafast route to manipulating quantum material properties<sup><CitationRef AdditionalCitationIDS="CR2 CR3 CR4" CitationID="CR1">1</CitationRef>–<CitationRef CitationID="CR5">5</CitationRef></sup>. Fractional Chern ferromagnetic states in moiré superlattices are a&#xa0;promising&#xa0;platform by which&#xa0;to pursue topological quantum computing<sup><CitationRef AdditionalCitationIDS="CR7 CR8 CR9" CitationID="CR6">6</CitationRef>–<CitationRef CitationID="CR10">10</CitationRef></sup>, but an effective optical control protocol has remained elusive. Here we demonstrate robust optical switching of integer and fractional Chern ferromagnets in twisted molybdenum ditelluride (MoTe<sub>2</sub>) bilayers using continuous-wave circularly polarized light. Highly efficient optical manipulation of spin orientations in the topological ferromagnet regime is realized at zero field using a pump light power as low as 28 nW µm<sup>−2</sup>. Using this optically induced transition, we also demonstrate magnetic bistate cycling and spatially resolved writing of ferromagnetic domain walls. This work establishes a reliable and efficient optical control scheme for moiré Chern ferromagnets, paving the way for dissipationless spintronics and quantized Chern junction devices.</p>

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Optical switching of a moiré Chern ferromagnet

  • Xiangbin Cai,
  • Haiyang Pan,
  • Yuzhu Wang,
  • Abdullah Rasmita,
  • Shunshun Yang,
  • Yan Zhao,
  • Wei Wang,
  • Ruihuan Duan,
  • Ruihua He,
  • Kenji Watanabe,
  • Takashi Taniguchi,
  • Zheng Liu,
  • Jesús Zúñiga-Pérez,
  • Bo Yang,
  • Weibo Gao

摘要

Optical control offers a non-contact, high-precision and ultrafast route to manipulating quantum material properties15. Fractional Chern ferromagnetic states in moiré superlattices are a promising platform by which to pursue topological quantum computing610, but an effective optical control protocol has remained elusive. Here we demonstrate robust optical switching of integer and fractional Chern ferromagnets in twisted molybdenum ditelluride (MoTe2) bilayers using continuous-wave circularly polarized light. Highly efficient optical manipulation of spin orientations in the topological ferromagnet regime is realized at zero field using a pump light power as low as 28 nW µm−2. Using this optically induced transition, we also demonstrate magnetic bistate cycling and spatially resolved writing of ferromagnetic domain walls. This work establishes a reliable and efficient optical control scheme for moiré Chern ferromagnets, paving the way for dissipationless spintronics and quantized Chern junction devices.