<p>The electronic quality of two-dimensional systems is crucial when exploring quantum transport phenomena. In semiconductor heterostructures, decades of optimization have yielded record-quality two-dimensional gases with transport and quantum mobilities reaching close to 10<sup>8</sup> and 10<sup>6</sup> cm<sup>2</sup> V<sup>−1</sup> s<sup>−1</sup>, respectively<sup><CitationRef AdditionalCitationIDS="CR2 CR3 CR4 CR5 CR6 CR7 CR8 CR9" CitationID="CR1">1</CitationRef>–<CitationRef CitationID="CR10">10</CitationRef></sup>. Although the quality of graphene devices has also been improving, it remains comparatively lower<sup><CitationRef AdditionalCitationIDS="CR12 CR13 CR14 CR15 CR16" CitationID="CR11">11</CitationRef>–<CitationRef CitationID="CR17">17</CitationRef></sup>. Here we report a transformative improvement in the electronic quality of graphene by employing graphite gates placed in its immediate proximity, at 1 nm separation. The resulting screening reduces charge inhomogeneity by two orders of magnitude, bringing it down to a few 10<sup>7</sup> cm<sup>−2</sup> and limiting potential fluctuations to less than 1 meV. Quantum mobilities reach 10<sup>7</sup> cm<sup>2</sup> V<sup>−1</sup> s<sup>−1</sup>, surpassing those in the highest-quality semiconductor heterostructures by an order of magnitude, and the transport mobilities match their record<sup><CitationRef CitationID="CR9">9</CitationRef>,<CitationRef CitationID="CR10">10</CitationRef></sup>. This quality enables Shubnikov–de Haas oscillations in fields as low as 1 mT and quantum Hall plateaux below 5 mT. Although proximity screening predictably suppresses electron–electron interactions, fractional quantum Hall states remain observable with their energy gaps reduced only by a factor of 3–5 compared with unscreened devices, demonstrating that many-body phenomena at spatial scales shorter than 10 nm remain robust. Our results offer a reliable route to improving electronic quality in graphene and other two-dimensional systems, which should facilitate the exploration of new physics previously obscured by disorder.</p>

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Proximity screening greatly enhances electronic quality of graphene

  • Daniil Domaretskiy,
  • Zefei Wu,
  • Van Huy Nguyen,
  • Ned Hayward,
  • Ian Babich,
  • Xiao Li,
  • Ekaterina Nguyen,
  • Julien Barrier,
  • Kornelia Indykiewicz,
  • Wendong Wang,
  • Roman V. Gorbachev,
  • Na Xin,
  • Kenji Watanabe,
  • Takashi Taniguchi,
  • Lee Hague,
  • Vladimir I. Fal’ko,
  • Irina V. Grigorieva,
  • Leonid A. Ponomarenko,
  • Alexey I. Berdyugin,
  • Andre K. Geim

摘要

The electronic quality of two-dimensional systems is crucial when exploring quantum transport phenomena. In semiconductor heterostructures, decades of optimization have yielded record-quality two-dimensional gases with transport and quantum mobilities reaching close to 108 and 106 cm2 V−1 s−1, respectively110. Although the quality of graphene devices has also been improving, it remains comparatively lower1117. Here we report a transformative improvement in the electronic quality of graphene by employing graphite gates placed in its immediate proximity, at 1 nm separation. The resulting screening reduces charge inhomogeneity by two orders of magnitude, bringing it down to a few 107 cm−2 and limiting potential fluctuations to less than 1 meV. Quantum mobilities reach 107 cm2 V−1 s−1, surpassing those in the highest-quality semiconductor heterostructures by an order of magnitude, and the transport mobilities match their record9,10. This quality enables Shubnikov–de Haas oscillations in fields as low as 1 mT and quantum Hall plateaux below 5 mT. Although proximity screening predictably suppresses electron–electron interactions, fractional quantum Hall states remain observable with their energy gaps reduced only by a factor of 3–5 compared with unscreened devices, demonstrating that many-body phenomena at spatial scales shorter than 10 nm remain robust. Our results offer a reliable route to improving electronic quality in graphene and other two-dimensional systems, which should facilitate the exploration of new physics previously obscured by disorder.