<p>The fractional quantum anomalous Hall (FQAH) effect was recently discovered in twisted MoTe<sub>2</sub> (tMoTe<sub>2</sub>) bilayers<sup><CitationRef AdditionalCitationIDS="CR2 CR3" CitationID="CR1">1</CitationRef>–<CitationRef CitationID="CR4">4</CitationRef></sup>. Experiments so far have revealed Chern insulators from hole doping at <i>ν</i> = −1, −2/3, −3/5 and −4/7 (per moiré unit cell)<sup><CitationRef AdditionalCitationIDS="CR2 CR3 CR4 CR5" CitationID="CR1">1</CitationRef>–<CitationRef CitationID="CR6">6</CitationRef></sup>. In parallel, theories predict that, between <i>v</i> = −1 and −3, there exist exotic quantum phases<sup><CitationRef AdditionalCitationIDS="CR8 CR9 CR10 CR11 CR12 CR13 CR14" CitationID="CR7">7</CitationRef>–<CitationRef CitationID="CR15">15</CitationRef></sup>, such as the coveted fractional topological insulators, fractional quantum spin Hall (FQSH) states and non-Abelian fractional states. Here we use transient optical spectroscopy<sup><CitationRef CitationID="CR16">16</CitationRef>,<CitationRef CitationID="CR17">17</CitationRef></sup> on tMoTe<sub>2</sub> to reveal nearly 20 hidden states at fractional fillings that are absent in static optical sensing or transport measurements. A pump pulse selectively excites charge across the correlated or pseudogaps, leading to the disordering (melting) of correlated states<sup><CitationRef CitationID="CR18">18</CitationRef></sup>. A probe pulse detects the subsequent melting and recovery dynamics by means of exciton and trion sensing<sup><CitationRef CitationID="CR1">1</CitationRef>,<CitationRef CitationID="CR3">3</CitationRef>,<CitationRef AdditionalCitationIDS="CR20" CitationID="CR19">19</CitationRef>–<CitationRef CitationID="CR21">21</CitationRef></sup>. Besides the known states, we observe further fractional fillings between <i>ν</i> = 0 and −1 and a large number of states on the electron doping side (<i>ν</i> &gt; 0). Most importantly, we observe new states at fractional fillings of the Chern bands at <i>ν</i> = −4/3, −3/2, −5/3, −7/3, −5/2 and −8/3. These states are potential candidates for the predicted exotic topological phases<sup><CitationRef AdditionalCitationIDS="CR8 CR9 CR10 CR11 CR12 CR13 CR14" CitationID="CR7">7</CitationRef>–<CitationRef CitationID="CR15">15</CitationRef></sup>. Moreover, we show that melting of correlated states occurs on two distinct timescales, 2–4 ps and 180–270 ps, attributed to electronic and phonon mechanisms, respectively. We discuss the differing dynamics of the electron-doped and hole-doped states from the distinct moiré conduction and valence bands.</p>

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Hidden states and dynamics of fractional fillings in twisted MoTe2 bilayers

  • Yiping Wang,
  • Jeongheon Choe,
  • Eric Anderson,
  • Weijie Li,
  • Julian Ingham,
  • Eric A. Arsenault,
  • Yiliu Li,
  • Xiaodong Hu,
  • Takashi Taniguchi,
  • Kenji Watanabe,
  • Xavier Roy,
  • Dmitri Basov,
  • Di Xiao,
  • Raquel Queiroz,
  • James C. Hone,
  • Xiaodong Xu,
  • X.-Y. Zhu

摘要

The fractional quantum anomalous Hall (FQAH) effect was recently discovered in twisted MoTe2 (tMoTe2) bilayers14. Experiments so far have revealed Chern insulators from hole doping at ν = −1, −2/3, −3/5 and −4/7 (per moiré unit cell)16. In parallel, theories predict that, between v = −1 and −3, there exist exotic quantum phases715, such as the coveted fractional topological insulators, fractional quantum spin Hall (FQSH) states and non-Abelian fractional states. Here we use transient optical spectroscopy16,17 on tMoTe2 to reveal nearly 20 hidden states at fractional fillings that are absent in static optical sensing or transport measurements. A pump pulse selectively excites charge across the correlated or pseudogaps, leading to the disordering (melting) of correlated states18. A probe pulse detects the subsequent melting and recovery dynamics by means of exciton and trion sensing1,3,1921. Besides the known states, we observe further fractional fillings between ν = 0 and −1 and a large number of states on the electron doping side (ν > 0). Most importantly, we observe new states at fractional fillings of the Chern bands at ν = −4/3, −3/2, −5/3, −7/3, −5/2 and −8/3. These states are potential candidates for the predicted exotic topological phases715. Moreover, we show that melting of correlated states occurs on two distinct timescales, 2–4 ps and 180–270 ps, attributed to electronic and phonon mechanisms, respectively. We discuss the differing dynamics of the electron-doped and hole-doped states from the distinct moiré conduction and valence bands.