<p>The interplay between nontrivial band topology and layered antiferromagnetism in MnBi<sub>2</sub>Te<sub>4</sub> has opened a new avenue for exploring topological phases of matter<sup><CitationRef AdditionalCitationIDS="CR2 CR3" CitationID="CR1">1</CitationRef>–<CitationRef CitationID="CR4">4</CitationRef></sup>. The quantum anomalous Hall effect<sup><CitationRef CitationID="CR5">5</CitationRef></sup> and axion insulator state<sup><CitationRef CitationID="CR6">6</CitationRef></sup> have been observed in odd and even number layers of MnBi<sub>2</sub>Te<sub>4</sub>, and the quantum metric nonlinear Hall effect<sup><CitationRef CitationID="CR7">7</CitationRef>,<CitationRef CitationID="CR8">8</CitationRef></sup> has been shown to exist in this topological antiferromagnet. The rich and complex antiferromagnetic spin dynamics in MnBi<sub>2</sub>Te<sub>4</sub> is expected to generate new quantum anomalous Hall phenomena that are absent in conventional ferromagnetic topological insulators, but experimental observations are still unknown. Here we fabricate a device of 7-septuple-layer MnBi<sub>2</sub>Te<sub>4</sub> covered with an AlO<sub><i>x</i></sub> capping layer, which enables the investigation of antiferromagnetic quantum anomalous Hall effect over wide parameter spaces. By tuning the gate voltage and perpendicular magnetic field, we uncover a cascade of quantum phase transitions that can be attributed to the influence of complex spin configurations on edge state transport. Furthermore, we find that an in-plane magnetic field enhances both the coercive field and the&#xa0;exchange gap of the surface state, in contrast to that in the&#xa0;ferromagnetic quantum anomalous Hall state. Combined with numerical simulations, we propose that these peculiar features arise from the spin flip and flop transitions that are inherent to a&#xa0;van der Waals antiferromagnet. The versatile tunability of the quantum anomalous Hall effect in MnBi<sub>2</sub>Te<sub>4</sub> paves the way for potential applications in topological antiferromagnetic spintronics<sup><CitationRef CitationID="CR9">9</CitationRef>,<CitationRef CitationID="CR10">10</CitationRef></sup>.</p>

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Antiferromagnetic quantum anomalous Hall effect under spin flips and flops

  • Zichen Lian,
  • Yongchao Wang,
  • Yongqian Wang,
  • Wen-Han Dong,
  • Yang Feng,
  • Zehao Dong,
  • Mangyuan Ma,
  • Shuai Yang,
  • Liangcai Xu,
  • Yaoxin Li,
  • Bohan Fu,
  • Yuetan Li,
  • Wanjun Jiang,
  • Yong Xu,
  • Chang Liu,
  • Jinsong Zhang,
  • Yayu Wang

摘要

The interplay between nontrivial band topology and layered antiferromagnetism in MnBi2Te4 has opened a new avenue for exploring topological phases of matter14. The quantum anomalous Hall effect5 and axion insulator state6 have been observed in odd and even number layers of MnBi2Te4, and the quantum metric nonlinear Hall effect7,8 has been shown to exist in this topological antiferromagnet. The rich and complex antiferromagnetic spin dynamics in MnBi2Te4 is expected to generate new quantum anomalous Hall phenomena that are absent in conventional ferromagnetic topological insulators, but experimental observations are still unknown. Here we fabricate a device of 7-septuple-layer MnBi2Te4 covered with an AlOx capping layer, which enables the investigation of antiferromagnetic quantum anomalous Hall effect over wide parameter spaces. By tuning the gate voltage and perpendicular magnetic field, we uncover a cascade of quantum phase transitions that can be attributed to the influence of complex spin configurations on edge state transport. Furthermore, we find that an in-plane magnetic field enhances both the coercive field and the exchange gap of the surface state, in contrast to that in the ferromagnetic quantum anomalous Hall state. Combined with numerical simulations, we propose that these peculiar features arise from the spin flip and flop transitions that are inherent to a van der Waals antiferromagnet. The versatile tunability of the quantum anomalous Hall effect in MnBi2Te4 paves the way for potential applications in topological antiferromagnetic spintronics9,10.