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A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy

  • Wendy J. Shaw,
  • Michelle K. Kidder,
  • Simon R. Bare,
  • Massimiliano Delferro,
  • James R. Morris,
  • Francesca M. Toma,
  • Sanjaya D. Senanayake,
  • Tom Autrey,
  • Elizabeth J. Biddinger,
  • Shannon Boettcher,
  • Mark E. Bowden,
  • Phillip F. Britt,
  • Robert C. Brown,
  • R. Morris Bullock,
  • Jingguang G. Chen,
  • Claus Daniel,
  • Peter K. Dorhout,
  • Rebecca A. Efroymson,
  • Kelly J. Gaffney,
  • Laura Gagliardi,
  • Aaron S. Harper,
  • David J. Heldebrant,
  • Oana R. Luca,
  • Maxim Lyubovsky,
  • Jonathan L. Male,
  • Daniel J. Miller,
  • Tanya Prozorov,
  • Robert Rallo,
  • Rachita Rana,
  • Robert M. Rioux,
  • Aaron D. Sadow,
  • Joshua A. Schaidle,
  • Lisa A. Schulte,
  • William A. Tarpeh,
  • Dionisios G. Vlachos,
  • Bryan D. Vogt,
  • Robert S. Weber,
  • Jenny Y. Yang,
  • Elke Arenholz,
  • Brett A. Helms,
  • Wenyu Huang,
  • James L. Jordahl,
  • Canan Karakaya,
  • Kourosh (Cyrus) Kian,
  • Jotheeswari Kothandaraman,
  • Johannes Lercher,
  • Ping Liu,
  • Deepika Malhotra,
  • Karl T. Mueller,
  • Casey P. O’Brien,
  • Robert M. Palomino,
  • Long Qi,
  • José A. Rodriguez,
  • Roger Rousseau,
  • Jake C. Russell,
  • Michele L. Sarazen,
  • David S. Sholl,
  • Emily A. Smith,
  • Michaela Burke Stevens,
  • Yogesh Surendranath,
  • Christopher J. Tassone,
  • Ba Tran,
  • William Tumas,
  • Krista S. Walton

摘要

Electrification to reduce or eliminate greenhouse gas emissions is essential to mitigate climate change. However, a substantial portion of our manufacturing and transportation infrastructure will be difficult to electrify and/or will continue to use carbon as a key component, including areas in aviation, heavy-duty and marine transportation, and the chemical industry. In this Roadmap, we explore how multidisciplinary approaches will enable us to close the carbon cycle and create a circular economy by defossilizing these difficult-to-electrify areas and those that will continue to need carbon. We discuss two approaches for this: developing carbon alternatives and improving our ability to reuse carbon, enabled by separations. Furthermore, we posit that co-design and use-driven fundamental science are essential to reach aggressive greenhouse gas reduction targets.