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High-temperature superconductivity with zero resistance and strange-metal behaviour in La3Ni2O7−δ

  • Yanan Zhang,
  • Dajun Su,
  • Yanen Huang,
  • Zhaoyang Shan,
  • Hualei Sun,
  • Mengwu Huo,
  • Kaixin Ye,
  • Jiawen Zhang,
  • Zihan Yang,
  • Yongkang Xu,
  • Yi Su,
  • Rui Li,
  • Michael Smidman,
  • Meng Wang,
  • Lin Jiao,
  • Huiqiu Yuan

摘要

Recent experimental observations have showed some signatures of superconductivity close to 80 K in La3Ni2O7 under pressure and have raised the hope of achieving high-temperature superconductivity in bulk nickelates. However, a zero-resistance state—a key characteristic of a superconductor—was not observed. Here we show that the zero-resistance state does exist in single crystals of La3Ni2O7−δ using a liquid pressure medium at up to 30 GPa. We also find that the system remains metallic under applied pressures, suggesting the absence of a metal–insulator transition proximate to the superconductivity. Moreover, analysis of the normal state T-linear resistance reveals a link between this strange-metal behaviour and superconductivity. The association between strange-metal behaviour and high-temperature superconductivity is very much in line with other classes of unconventional superconductors, including the cuprates and Fe-based superconductors. Further investigations exploring the interplay of strange-metal behaviour and superconductivity, as well as possible competing electronic or structural phases, are essential to understand the mechanism of superconductivity in this system.