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A high-efficiency programmable modulator for extreme ultraviolet light with nanometre feature size based on an electronic phase transition

  • Igor Vaskivskyi,
  • Anze Mraz,
  • Rok Venturini,
  • Gregor Jecl,
  • Yevhenii Vaskivskyi,
  • Riccardo Mincigrucci,
  • Laura Foglia,
  • Dario De Angelis,
  • Jacopo-Stefano Pelli-Cresi,
  • Ettore Paltanin,
  • Danny Fainozzi,
  • Filippo Bencivenga,
  • Claudio Masciovecchio,
  • Dragan Mihailovic

摘要

The absence of efficient light modulators for extreme ultraviolet (EUV) and X-ray photons considerably limits their real-life application, particularly when even slight complexity of the beam patterns is required. Here we report on a novel approach to reversible imprinting of a holographic mask in an electronic Wigner crystal material with a sub-90-nm feature size. The structure is imprinted on a sub-picosecond timescale using EUV laser pulses, and acts as a high-efficiency diffraction grating that deflects EUV or soft X-ray light. The imprinted nanostructure is stable after the removal of the exciting beams at low temperatures, but can be easily erased by a single heating beam. Modelling shows that the efficiency of the device can exceed 1%, approaching state-of-the-art etched gratings, but with the benefit of being programmable and tunable over a large range of wavelengths. The observed effect is based on the rapid change of lattice constant upon transition between metastable electronically ordered phases in a layered transition metal dichalcogenide. The proposed approach is potentially useful for creating tunable light modulators in the EUV and soft X-ray spectral ranges.