<p>The interplay of strong electronic correlations, sizable octahedral distortions, and pronounced spin-orbit coupling (SOC) makes perovskite oxides promising candidates for realizing altermagnetic phases. We study altermagnetic phases in Ca<sub>3</sub>Ru<sub>2</sub>O<sub>7</sub>, a non-centrosymmetric layered perovskite whose ground state is a Kramers-degenerate antiferromagnet. We show that an alternative Néel-type spin arrangement hosts a P-2 <i>d</i>-wave altermagnetic state with orbital selectivity similar to Ca<sub>2</sub>RuO<sub>4</sub>. Including SOC generates a symmetry-allowed <i>p</i>-wave component and yields a hybrid <i>d</i>/<i>p</i>-wave altermagnetic order. We further demonstrate that biaxial strain tunes both magnetic stability and band splitting: compressive strain beyond 2% favors the altermagnetic phase over the antiferromagnetic ground state, while tensile strain increases altermagnetic splittings by up to 9%. To quantify these trends, we define an altermagnetic figure of merit and trace its strain dependence to changes in electronic localization and octahedral geometry in this polar metal.</p>

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Hybrid d/p-wave altermagnetism in Ca3Ru2O7 and strain-controlled spin splitting

  • Andrea León,
  • Carmine Autieri,
  • Thomas Brumme,
  • Jhon W. González

摘要

The interplay of strong electronic correlations, sizable octahedral distortions, and pronounced spin-orbit coupling (SOC) makes perovskite oxides promising candidates for realizing altermagnetic phases. We study altermagnetic phases in Ca3Ru2O7, a non-centrosymmetric layered perovskite whose ground state is a Kramers-degenerate antiferromagnet. We show that an alternative Néel-type spin arrangement hosts a P-2 d-wave altermagnetic state with orbital selectivity similar to Ca2RuO4. Including SOC generates a symmetry-allowed p-wave component and yields a hybrid d/p-wave altermagnetic order. We further demonstrate that biaxial strain tunes both magnetic stability and band splitting: compressive strain beyond 2% favors the altermagnetic phase over the antiferromagnetic ground state, while tensile strain increases altermagnetic splittings by up to 9%. To quantify these trends, we define an altermagnetic figure of merit and trace its strain dependence to changes in electronic localization and octahedral geometry in this polar metal.