<p>Electrical control of magnetization in nanoscale devices can be significantly improved through the efficient generation of orbital currents and their conversion into spin currents. In nonmagnetic/ferromagnetic bilayers, this conversion produces a torque on the magnetization, enabling magnetization switching and dynamic manipulation. While previous studies focus on metallic ferromagnets, we demonstrate a large orbital torque and enhanced orbital-to-spin conversion by an antiferromagnetic insulating CoO layer. Measurements in CuO<sub>x</sub>/CoO/Co trilayers show that inserting CoO reverses the torque’s sign and triples its magnitude compared to CuO<sub>x</sub>/Co. This behaviour stems from the inverted oxygen gradient at the CuO<sub>x</sub>/CoO interface and CoO’s high orbital multiplicity, which favours the transmission of orbital momenta and efficient orbital-to-spin conversion. At low temperatures, the onset of antiferromagnetic order induces a further many-fold increase of the torque, which we attribute to the efficient excitation and propagation of spin-orbit excitons induced by magnetic coupling. Comparative measurements of CuO<sub>x</sub>/NiO/Co and CuO<sub>x</sub>/MnO/Co trilayers show that the torque efficiency scales with the orbital momentum of the Co<sup>2+</sup>, Ni<sup>2+</sup>, and Mn<sup>2+</sup> ions in the antiferromagnet. These results reveal that antiferromagnetic insulators like CoO provide highly effective orbital-to-spin transduction, combining orbital torque and exchange bias functionalities to improve the performance of spintronic devices.</p>

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Generation, transmission, and conversion of orbital torque by an antiferromagnetic insulator

  • Shilei Ding,
  • Paul Noël,
  • Gunasheel Kauwtilyaa Krishnaswamy,
  • Niccolò Davitti,
  • Giacomo Sala,
  • Marzia Fantauzzi,
  • Antonella Rossi,
  • Pietro Gambardella

摘要

Electrical control of magnetization in nanoscale devices can be significantly improved through the efficient generation of orbital currents and their conversion into spin currents. In nonmagnetic/ferromagnetic bilayers, this conversion produces a torque on the magnetization, enabling magnetization switching and dynamic manipulation. While previous studies focus on metallic ferromagnets, we demonstrate a large orbital torque and enhanced orbital-to-spin conversion by an antiferromagnetic insulating CoO layer. Measurements in CuOx/CoO/Co trilayers show that inserting CoO reverses the torque’s sign and triples its magnitude compared to CuOx/Co. This behaviour stems from the inverted oxygen gradient at the CuOx/CoO interface and CoO’s high orbital multiplicity, which favours the transmission of orbital momenta and efficient orbital-to-spin conversion. At low temperatures, the onset of antiferromagnetic order induces a further many-fold increase of the torque, which we attribute to the efficient excitation and propagation of spin-orbit excitons induced by magnetic coupling. Comparative measurements of CuOx/NiO/Co and CuOx/MnO/Co trilayers show that the torque efficiency scales with the orbital momentum of the Co2+, Ni2+, and Mn2+ ions in the antiferromagnet. These results reveal that antiferromagnetic insulators like CoO provide highly effective orbital-to-spin transduction, combining orbital torque and exchange bias functionalities to improve the performance of spintronic devices.