Abstract <p>The escalating environmental concerns regarding plastic waste necessitate innovative strategies for waste management and resource utilization. This study presents a novel approach for synthesizing high surface area activated carbon (AC) through a single-step process, using polyethylene terephthalate (PET) plastic waste as the precursor and potassium hydroxide (KOH) as the activating agent. The optimal activation conditions were established using a weight ratio of 1:1 of PET to KOH and annealing for 15&#xa0;min at 700&#xa0;°C. The conversion efficiency of PET plastic trash into AC exceeded 20%. The materials underwent thorough characterization using scanning electron microscopy (SEM), X-ray diffraction (XRD), Brunauer–Emmett–Teller (BET) analysis, and Fourier transform infrared spectroscopy (FTIR). The AC obtained has a mesoporous structure and a surface area of 1831.166 m<sup>2</sup>/g. The AC derived from plastic waste demonstrated excellent efficiency in removing organic dyes from aqueous solutions, achieving a maximum adsorption capacity of 131.58&#xa0;mg/g. The successful transformation of plastic waste into a valuable resource underscores the importance of innovative approaches to mitigating environmental degradation. The synthesized AC’s efficacy in adsorption-based remediation strategies demonstrates its potential for addressing various pollution issues and opens new avenues for valuing plastic waste.</p> Graphical Abstract <p></p> Highlights <p><UnorderedList Mark="Bullet"> <ItemContent> <p>PET plastic waste was converted into high-surface-area activated carbon using a single-step process.</p> </ItemContent> <ItemContent> <p>A surface area of 1831.166 m<sup>2</sup>/g was achieved, enhancing adsorption efficiency for pollutants.</p> </ItemContent> <ItemContent> <p>Activated carbon removed MB with a maximum adsorption capacity of 131.58 mg/g.</p> </ItemContent> <ItemContent> <p>SEM, XRD, BET, and FTIR were used to confirm the porous structure and chemical properties.</p> </ItemContent> <ItemContent> <p>A sustainable waste-to-resource approach was demonstrated for environmental remediation.</p> </ItemContent> </UnorderedList></p>

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Single-step Synthesis of High Surface Area Activated Carbon from Polyethylene Terephthalate Plastic Waste for Environmental Treatment Applications

  • Hoan Thi Lai,
  • Quoc Anh Le,
  • Nga Thuy Tran,
  • Chinh Van Tran,
  • Phuong Hien Ho,
  • D. Duc Nguyen,
  • H. Phuong Nguyen Thi,
  • Duong Duc La

摘要

Abstract

The escalating environmental concerns regarding plastic waste necessitate innovative strategies for waste management and resource utilization. This study presents a novel approach for synthesizing high surface area activated carbon (AC) through a single-step process, using polyethylene terephthalate (PET) plastic waste as the precursor and potassium hydroxide (KOH) as the activating agent. The optimal activation conditions were established using a weight ratio of 1:1 of PET to KOH and annealing for 15 min at 700 °C. The conversion efficiency of PET plastic trash into AC exceeded 20%. The materials underwent thorough characterization using scanning electron microscopy (SEM), X-ray diffraction (XRD), Brunauer–Emmett–Teller (BET) analysis, and Fourier transform infrared spectroscopy (FTIR). The AC obtained has a mesoporous structure and a surface area of 1831.166 m2/g. The AC derived from plastic waste demonstrated excellent efficiency in removing organic dyes from aqueous solutions, achieving a maximum adsorption capacity of 131.58 mg/g. The successful transformation of plastic waste into a valuable resource underscores the importance of innovative approaches to mitigating environmental degradation. The synthesized AC’s efficacy in adsorption-based remediation strategies demonstrates its potential for addressing various pollution issues and opens new avenues for valuing plastic waste.

Graphical Abstract

Highlights

PET plastic waste was converted into high-surface-area activated carbon using a single-step process.

A surface area of 1831.166 m2/g was achieved, enhancing adsorption efficiency for pollutants.

Activated carbon removed MB with a maximum adsorption capacity of 131.58 mg/g.

SEM, XRD, BET, and FTIR were used to confirm the porous structure and chemical properties.

A sustainable waste-to-resource approach was demonstrated for environmental remediation.