<p>Organic solar cells (OSCs) have experienced remarkable performance progress up to 20% benchmark power conversion efficiency (PCE) in past years. Considering the &lt;1% initial PCE obtained by OSC decades ago, the milestone of surpassing 20% efficiency is of great significance. Meanwhile, further performance promotion is urgently required for OSCs as other solution-processable photovoltaic technologies are also competitive. This review article aims to demonstrate a comprehensive summary of recent reports on OSCs with over 20% PCE, delving into key strategies including material innovations, multi-component system construction, deposition protocol optimization, solid/solvent additive engineering, as well as hole/electron transport layer development. In addition, this study identifies the next-stage scientific and technological issues that warrant greater attention. These issues are proposed to drive more prosperous research development, particularly in the field of flexible and wearable power suppliers.</p>

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Organic solar cells: beyond 20%

  • Ruijie Ma,
  • Zhenghui Luo,
  • Youdi Zhang,
  • Lingling Zhan,
  • Tao Jia,
  • Pei Cheng,
  • Cenqi Yan,
  • Qunping Fan,
  • Shengjian Liu,
  • Long Ye,
  • Guangye Zhang,
  • Xiaopeng Xu,
  • Wei Gao,
  • Yue Wu,
  • Jiaying Wu,
  • Yuxiang Li,
  • Yuhang Liu,
  • Feng Liu,
  • Jiali Song,
  • Haiyang Chen,
  • Weijie Chen,
  • Xin Zhang,
  • Yahui Liu,
  • Jun Yuan,
  • Quan Liu,
  • Zhipeng Kan,
  • Hang Yin,
  • Xiaojun Li,
  • Yunlong Ma,
  • Dan Deng,
  • Lei Zhu,
  • Yong Huo,
  • Baobin Fan,
  • Huiting Fu,
  • Xunfan Liao,
  • Hanlin Hu,
  • Chao Li,
  • Runnan Yu,
  • Huawei Hu,
  • Zhaoyang Yao,
  • Yunhao Cai,
  • Deping Qian,
  • Yong Cui,
  • Huifeng Yao,
  • Bowei Xu,
  • Bin Kan,
  • Ke Gao,
  • Chunhui Duan,
  • Xiaotian Hu,
  • Huiliang Sun

摘要

Organic solar cells (OSCs) have experienced remarkable performance progress up to 20% benchmark power conversion efficiency (PCE) in past years. Considering the <1% initial PCE obtained by OSC decades ago, the milestone of surpassing 20% efficiency is of great significance. Meanwhile, further performance promotion is urgently required for OSCs as other solution-processable photovoltaic technologies are also competitive. This review article aims to demonstrate a comprehensive summary of recent reports on OSCs with over 20% PCE, delving into key strategies including material innovations, multi-component system construction, deposition protocol optimization, solid/solvent additive engineering, as well as hole/electron transport layer development. In addition, this study identifies the next-stage scientific and technological issues that warrant greater attention. These issues are proposed to drive more prosperous research development, particularly in the field of flexible and wearable power suppliers.