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High-quality crystalline NiO/β-Ga2O3 p–n heterojunctions grown by the low-cost and vacuum-free mist-CVD for device applications

  • Zeyulin Zhang,
  • Qingwen Song,
  • Dinghe Liu,
  • Yiru Yan,
  • Hao Chen,
  • Changgen Mu,
  • Dazheng Chen,
  • Qian Feng,
  • Jincheng Zhang,
  • Yuming Zhang,
  • Yue Hao,
  • Chunfu Zhang

摘要

Gallium oxide (Ga2O3) p–n heterojunctions play an important role in addressing the difficulties in Ga2O3 p-type doping. Therefore, an efficient and economical fabrication method needs to be established to create single-crystal Ga2O3 heterojunctions for device applications. In this work, we successfully achieved epitaxial growth of single-crystal nickel oxide (NiO) and β-Ga2O3 heterojunctions based on the low-cost and vacuum-free mist chemical-vapor deposition. The full width at half maximum of the X-ray diffraction rocking curves of NiO (111) and β-Ga2O3 (−201) reached 0.077° and 0.807°, respectively. The energy band between NiO and β-Ga2O3 has a Type II heterojunction. Finally, we prepared a quasi-vertical diode based on the NiO/β-Ga2O3 heterojunction, which exhibits obvious rectification characteristics of the p–n junction and provides a reverse breakdown voltage of 117 V. This work proposes a low-cost fabrication method for β-Ga2O3 p–n heterojunctions.