Data-driven insights into the high-temperature behavior of polymer/carbon nanotubes nanocomposites
摘要
In this study, the hardness and tensile strength of polypropylene/carbon nanotubes (PP/CNT) and low-density polyethylene/carbon nanotubes (LDPE/CNT) composite materials were predicted using machine learning (ML). The composites were fabricated through a microwave-assisted manufacturing process, and their mechanical properties were evaluated at an elevated temperature of 100 °C, which remains below the melting points of both PP and LDPE. Hardness and tensile tests were conducted using a Rockwell hardness tester and a universal testing machine, respectively. To predict these properties, various ML algorithms, i.e., extreme gradient boosting (XGBoost), K-nearest neighbors (KNN), and random forest (RF), were employed. Among these, the RF model demonstrated the highest accuracy and consistency, particularly for PP/CNT composites. Performance metrics, including root mean square error (RMSE), mean absolute error (MAE), and coefficient of determination (R2), indicated that the RF model outperformed other algorithms. For PP/CNT composites, it exhibited minimal variations of ± 0.5 for hardness and ± 2 for tensile strength, highlighting strong predictive accuracy. In contrast, LDPE/CNT composites showed greater variations of ± 1 and ± 3, respectively, due to a weaker correlation between predicted and experimental values. Overall, this study underscores the potential of ML, particularly the RF algorithm, in providing reliable predictions of composite material properties.
Graphical abstract