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pH-responsive corrosion protection of chitosan-coated hollow mesoporous silica microspheres loaded with 2-mercaptobenzothiazole coating on copper substrates

  • Gui-wen Chu,
  • Zhi-hao Wang,
  • Hao-ran Zhang,
  • Peng Wu,
  • Jian-kai Zhang,
  • Hao Shi,
  • Li-ying Song,
  • Fu-bin Ma,
  • Qiang Sun,
  • Zhan Gao,
  • Yi-xiang Wang,
  • Lei Sun,
  • Zi-chen Cao

摘要

An active protection coating for pH-responsive was prepared. The hollow mesoporous silica microspheres (HMSNs) were loaded with 2-mercaptobenzothiazole (MBT), and then they were coated with chitosan (CS). The composite microspheres were in the range of 650–750 nm in diameter. CS-HMSN-MBT coating had a faster repair rate under acidic conditions by synergistic effect between CS and MBT. The repair rate under alkaline conditions was slowed down. The active protection performance reached the strongest after 3 d immersion. The corrosion inhibitor release mechanism was optimized to extend the service life of the coating and to achieve long-term service of the copper substrate.