<p>We propose a 2D graphene structure containing atomic ensemble as a platform for implementing nanoscale enhanced coherent interactions of plasmonic fields with resonant atomic systems. We determine the graphene surface plasmon modes, the properties of its electromagnetic fields, and emphasize the role of graphene sheet separation on the interaction with atomic systems for various dipole orientations and positions between the graphene sheets. We analyze the conditions for implementation of nanoscale coherent interaction of surface plasmon mode with resonant atomic ensembles. By solving the Maxwell-Bloch equations that govern the resonant interaction of surface plasmons with atoms, we derive the modified area theorem, which makes it possible to identify the most common nonlinear patterns in the behavior of plasmons under the studied conditions. We obtain analytical and numerical solutions of the area theorem and find the possibility of stable propagation of isolated pulses of graphene surface plasmon modes at “fractional” pulse area values relative to <InlineEquation ID="IEq1"> <EquationSource Format="TEX">\(\pi \)</EquationSource> <EquationSource Format="MATHML"><math> <mi>π</mi> </math></EquationSource> </InlineEquation>. We show that the coherent dynamics of surface plasmon fields can be realized in nanoscale design, and highlight the possibilities of using this scheme of coherent dynamics for implementing compact multimode nanoscale quantum memory and its integration with other quantum devices on the proposed platform.</p>