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<p>In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials is how the electron correlation manifests and interacts with the magnetic orders. In this study, we demonstrate that the recently discovered 2D antiferromagnetic material, CrSBr is a Mott insulator, through the combined use of resonant and temperature-dependent angle-resolved photoemission spectroscopy techniques, supplemented by dynamical mean-field theory analysis. Intriguingly, we found that as the system transitions from the antiferromagnetic to the paramagnetic phases, its Mott bands undergo a reconfiguration, and a coherent-incoherent crossover, driven by the dissolution of the magnetic order. Our findings reveal a distinctive evolution of band structure associated with magnetic phase transitions, shedding light on the investigation of the intricate interplay between correlation and magnetic orders in strongly correlated van der Waals magnetic materials.</p>

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Mott insulating phase and coherent-incoherent crossover across magnetic phase transition in 2D antiferromagnetic CrSBr

  • 期刊论文

  • 发表日期：

    2025年3月19日

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  • Fan Wu,
  • Xuefeng Zhang,
  • Yi Chen,
  • Ding Pei,
  • Mengwen Zhan,
  • Zicheng Tao,
  • Cheng Chen,
  • Shipeng Lu,
  • Jingzhi Chen,
  • Shujie Tang,
  • Xia Wang,
  • Yanfeng Guo,
  • Lexian Yang,
  • Yan Zhang,
  • Yulin Chen,
  • Qixi Mi,
  • Gang Li,
  • Zhongkai Liu

摘要

In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials is how the electron correlation manifests and interacts with the magnetic orders. In this study, we demonstrate that the recently discovered 2D antiferromagnetic material, CrSBr is a Mott insulator, through the combined use of resonant and temperature-dependent angle-resolved photoemission spectroscopy techniques, supplemented by dynamical mean-field theory analysis. Intriguingly, we found that as the system transitions from the antiferromagnetic to the paramagnetic phases, its Mott bands undergo a reconfiguration, and a coherent-incoherent crossover, driven by the dissolution of the magnetic order. Our findings reveal a distinctive evolution of band structure associated with magnetic phase transitions, shedding light on the investigation of the intricate interplay between correlation and magnetic orders in strongly correlated van der Waals magnetic materials.