Zeolite-based materials for greenhouse gas capture and conversion
摘要
The global warming caused by greenhouse gas emissions, principally carbon dioxide (CO2) and methane (CH4), has become a great threat to human survival. The capture and conversion of CO2 and CH4 not only provide an effective method to reduce the greenhouse gas emissions towards achieving carbon neutrality but also produce sustainable chemicals and fuels to meet the increasing demand for chemicals and energy. Zeolite-based materials are excellent adsorbents and catalysts for CO2 and CH4 capture and conversion. In this mini-review, we present the recent progress in zeolite-based materials for CO2 and CH4 capture and conversion. We first discuss the key factors of zeolites on the CO2 and CH4 adsorption performance. Then, we demonstrate the catalytic conversion of CO2 and CH4 into value-added chemicals, including hydrocarbons, oxygenates, and syngas. Finally, we provide an outlook regarding the opportunities and challenges for the capture and conversion of CO2 and CH4 towards achieving carbon neutrality and sustainable development.