Adiabatic tapered silica optical nanofibers: optimized design for entangled quantum states generation
摘要
Spontaneous parametric down-conversion (SPDC) is a fundamental nonlinear optical mechanism that generates entangled photon pairs, serving as a primary source of entangled quantum states in quantum optics. Silica tapered optical fibers (TOFs), despite their weaker effective second-order nonlinearity compared with non-centrosymmetric crystals, offer a compact, low-loss, all-fiber SPDC platform due to strong optical confinement and long interaction lengths. Their effective second-order response originates from surface dipole and bulk multipole contributions induced by subwavelength symmetry breaking. In this paper, we conduct a theoretical analysis of a fully adiabatic silica TOF optimized for efficient generation of photon pairs forming entangled quantum states via SPDC, including both nonlinear contributions. The effective second-order nonlinear susceptibility can be further enhanced via functionalization with nonlinear molecular layers deposited solely on the nanofiber waist, significantly improving entangled quantum state generation without affecting taper propagation. Adiabatic control of light propagation through the two taper transitions is shown to be essential for maximizing generation efficiency. An adiabaticity criterion is introduced to establish an upper limit on the taper slope to ensure lossless coupling between the untapered fiber and the nanofiber section. The input taper is designed to remain adiabatic for the pump mode (HE21 or TM