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<p>This work reports a novel method for enhancing solar energy applications by synthesizing high-performance nanostructured PPy@AF hydrogel as photocatalyst under controlled conditions. The incorporation of acid fuchsin (AF) as a dopant into polypyrrole (PPy) imparts unique supramolecular properties to the hydrogels, enabling efficient chemical transformations, including C-H bond activation. The incorporation of AF as a dopant into PPy imparts unique supramolecular properties to the hydrogels, enabling efficient chemical transformations, including C-H bond activation. These dopant-enhanced hydrogel frameworks exhibit superior catalytic efficiency, offering a sustainable and eco-friendly solution for energy conversion processes. The study highlights the synergistic impact of dopant inclusion in enhancing the stability, selectivity, and reaction kinetics of the hydrogels. This innovation has the potential to contribute to the development of advanced materials in solar energy systems, where efficient catalytic reactions are essential. Overall, the findings support the advancement of high-performance, dopant-modified nanostructured hydrogels with promising applications in renewable energy and green chemistry.</p><p></p>

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Empowering solar energy: controlled synthesis of high-performance nanostructured hydrogel through dopant-enabled supramolecule innovation for organic transformations

  • 期刊论文

  • 发表日期：

    2025年10月6日

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  • Minakshi Chaudhary,
  • Rajesh K. Yadav,
  • Rehana Shahin,
  • Shaifali Mishra,
  • Kanchan Sharma,
  • Surendra K. Jaiswal,
  • Arun Kumar Dubey,
  • D. K. Dwivedi,
  • Alok Kumar Singh,
  • Jin-Ook Baeg

摘要

This work reports a novel method for enhancing solar energy applications by synthesizing high-performance nanostructured PPy@AF hydrogel as photocatalyst under controlled conditions. The incorporation of acid fuchsin (AF) as a dopant into polypyrrole (PPy) imparts unique supramolecular properties to the hydrogels, enabling efficient chemical transformations, including C-H bond activation. The incorporation of AF as a dopant into PPy imparts unique supramolecular properties to the hydrogels, enabling efficient chemical transformations, including C-H bond activation. These dopant-enhanced hydrogel frameworks exhibit superior catalytic efficiency, offering a sustainable and eco-friendly solution for energy conversion processes. The study highlights the synergistic impact of dopant inclusion in enhancing the stability, selectivity, and reaction kinetics of the hydrogels. This innovation has the potential to contribute to the development of advanced materials in solar energy systems, where efficient catalytic reactions are essential. Overall, the findings support the advancement of high-performance, dopant-modified nanostructured hydrogels with promising applications in renewable energy and green chemistry.