<p>This paper details the experimental development of a Cryogenic Tracer Irradiation Facility (CTIF) at the University of Texas at Austin (UT Austin). UT Austin produces gaseous radiotracers with in-core facilities, but an ex-core facility is possible using a helium compressor to freeze the target. A sample of natural xenon was irradiated using this method. The neutron flux was calculated to be 5.13 ∗ 10<sup>11</sup> ± 3.94% neutrons/cm<sup>2</sup>/s for a reactor power of 900&#xa0;kW. Assuming a one-hour irradiation at the same reactor power with one liter at STP of <sup>126</sup>Xe, the CTIF produced 3.62 ∗ 10<sup>7</sup> ± 3.94% Bq of <sup>127</sup>Xe at the end of irradiation. The production rate for xenon isotopes in the cryogenic irradiation facility in the reactor beam port is found to be approximately 10% of the reaction rate in the previously demonstrated in-core irradiation facility. The cryogenic facility will be an excellent candidate for producing radioxenon isotopes on the order of 100&#xa0;mCi (3.7 × 10<sup>9</sup>&#xa0;Bq), but will not match the production rate of the in-core production method. Placing such a facility in a beam port with a higher flux provides a promising path forward.</p>

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Production of gaseous radiotracers with a cryogenic irradiation facility

  • Clayton Hudson,
  • Joseph Lapka,
  • Johnathan Slack,
  • Christine Johnson,
  • Carolyn Seifert,
  • Derek Haas

摘要

This paper details the experimental development of a Cryogenic Tracer Irradiation Facility (CTIF) at the University of Texas at Austin (UT Austin). UT Austin produces gaseous radiotracers with in-core facilities, but an ex-core facility is possible using a helium compressor to freeze the target. A sample of natural xenon was irradiated using this method. The neutron flux was calculated to be 5.13 ∗ 1011 ± 3.94% neutrons/cm2/s for a reactor power of 900 kW. Assuming a one-hour irradiation at the same reactor power with one liter at STP of 126Xe, the CTIF produced 3.62 ∗ 107 ± 3.94% Bq of 127Xe at the end of irradiation. The production rate for xenon isotopes in the cryogenic irradiation facility in the reactor beam port is found to be approximately 10% of the reaction rate in the previously demonstrated in-core irradiation facility. The cryogenic facility will be an excellent candidate for producing radioxenon isotopes on the order of 100 mCi (3.7 × 109 Bq), but will not match the production rate of the in-core production method. Placing such a facility in a beam port with a higher flux provides a promising path forward.