<p>Stable isotope taggants added to nuclear materials could be utilized as diagnostic nuclear forensics signatures; however, intentionally adding taggants is a relatively new and untested concept with respect to the nuclear fuel cycle. In this study, we added trace amounts of stable Mo and W isotope taggants to starting materials used to synthesize UO<sub>2</sub> along a wet synthesis pathway. Successful incorporation and recovery of the Mo and W taggants was achieved in the UO<sub>2</sub> product and all its precursors. This study demonstrates the efficacy of stable isotope tagging along a wet UO<sub>2</sub> production pathway.</p>

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Recovery of stable isotope taggants along a wet production pathway of uranium dioxide

  • Quinn R. Shollenberger,
  • Jan Render,
  • Aaron Chalifoux,
  • Miguel Cisneros,
  • Naomi Marks,
  • Luther McDonald,
  • John M. Rolison

摘要

Stable isotope taggants added to nuclear materials could be utilized as diagnostic nuclear forensics signatures; however, intentionally adding taggants is a relatively new and untested concept with respect to the nuclear fuel cycle. In this study, we added trace amounts of stable Mo and W isotope taggants to starting materials used to synthesize UO2 along a wet synthesis pathway. Successful incorporation and recovery of the Mo and W taggants was achieved in the UO2 product and all its precursors. This study demonstrates the efficacy of stable isotope tagging along a wet UO2 production pathway.