<p>This study introduces a novel application of radiochronometry to estimate nuclide inventories in molten salt reactor off-gas systems based on gamma spectroscopic data from the Molten Salt Reactor Experiment. By analyzing isotopic, isobaric, and isomeric activity ratios, key depletion model parameters related to species transport within the reactor system could be inferred. The findings demonstrate the potential of leveraging a limited subset of gamma spectroscopy measurements to accurately estimate nuclide inventories throughout the off-gas system. The approach can be useful in reactor design activities and support analyses relevant to operations, safety, security, and safeguards.</p>

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Radiochemical transport analysis of gamma spectroscopic data to support estimation of molten salt reactor off-gas inventories

  • Shayan Shahbazi,
  • Tingzhou Fei

摘要

This study introduces a novel application of radiochronometry to estimate nuclide inventories in molten salt reactor off-gas systems based on gamma spectroscopic data from the Molten Salt Reactor Experiment. By analyzing isotopic, isobaric, and isomeric activity ratios, key depletion model parameters related to species transport within the reactor system could be inferred. The findings demonstrate the potential of leveraging a limited subset of gamma spectroscopy measurements to accurately estimate nuclide inventories throughout the off-gas system. The approach can be useful in reactor design activities and support analyses relevant to operations, safety, security, and safeguards.