<p>The optical properties of the superconducting K<InlineEquation ID="IEq11"> <EquationSource Format="TEX">\(_{0.8}\)</EquationSource> </InlineEquation>Fe<InlineEquation ID="IEq12"> <EquationSource Format="TEX">\(_{1.7}\)</EquationSource> </InlineEquation>(Se<InlineEquation ID="IEq13"> <EquationSource Format="TEX">\(_{0.73}\)</EquationSource> </InlineEquation>S<InlineEquation ID="IEq14"> <EquationSource Format="TEX">\(_{0.27}\)</EquationSource> </InlineEquation>)<InlineEquation ID="IEq15"> <EquationSource Format="TEX">\(_2\)</EquationSource> </InlineEquation> single crystals with a critical temperature <InlineEquation ID="IEq16"> <EquationSource Format="TEX">\(T_c\approx 26\)</EquationSource> </InlineEquation> K have been measured in the <i>ab</i> plane in a wide frequency range using both infrared Fourier-transform spectroscopy and spectroscopic ellipsometry at temperatures of 4–300 K. The normal-state reflectance of K<InlineEquation ID="IEq17"> <EquationSource Format="TEX">\(_{0.8}\)</EquationSource> </InlineEquation>Fe<InlineEquation ID="IEq18"> <EquationSource Format="TEX">\(_{1.7}\)</EquationSource> </InlineEquation>(Se<InlineEquation ID="IEq19"> <EquationSource Format="TEX">\(_{0.73}\)</EquationSource> </InlineEquation>S<InlineEquation ID="IEq20"> <EquationSource Format="TEX">\(_{0.27}\)</EquationSource> </InlineEquation>)<InlineEquation ID="IEq21"> <EquationSource Format="TEX">\(_2\)</EquationSource> </InlineEquation> is analyzed using a Drude-Lorentz model with one Drude component. The temperature dependences of the plasma frequency, optical conductivity, scattering rate, and dc resistivity of the Drude contribution in the normal state are presented. In the superconducting state, we observe a signature of the superconducting gap opening at <InlineEquation ID="IEq22"> <EquationSource Format="TEX">\(2\Delta (0)=11.8\)</EquationSource> </InlineEquation>&#xa0;meV. An abrupt decrease in the low-frequency dielectric permittivity <InlineEquation ID="IEq23"> <EquationSource Format="TEX">\(\varepsilon _1(\omega )\)</EquationSource> </InlineEquation> at <InlineEquation ID="IEq24"> <EquationSource Format="TEX">\(T &lt; T_c\)</EquationSource> </InlineEquation> also evidences the formation of the superconducting condensate. The superconducting plasma frequency <InlineEquation ID="IEq25"> <EquationSource Format="TEX">\(\omega _{pl,s} = (213\pm 5)\)</EquationSource> </InlineEquation>&#xa0;cm<InlineEquation ID="IEq26"> <EquationSource Format="TEX">\(^{-1}\)</EquationSource> </InlineEquation> and the magnetic penetration depth <InlineEquation ID="IEq27"> <EquationSource Format="TEX">\(\lambda =(7.5\pm 0.2)\)</EquationSource> </InlineEquation>&#xa0;<InlineEquation ID="IEq28"> <EquationSource Format="TEX">\(\mu\)</EquationSource> </InlineEquation>m are determined.</p>

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Optical Properties of Superconducting K\(_{0.8}\)Fe\(_{1.7}\)(Se\(_{0.73}\)S\(_{0.27}\))\(_2\) Single Crystals

  • Andrei Muratov,
  • Yevgeny Rakhmanov,
  • Andrei Shilov,
  • Igor Morozov,
  • Yurii Aleshchenko

摘要

The optical properties of the superconducting K \(_{0.8}\) Fe \(_{1.7}\) (Se \(_{0.73}\) S \(_{0.27}\) ) \(_2\) single crystals with a critical temperature \(T_c\approx 26\) K have been measured in the ab plane in a wide frequency range using both infrared Fourier-transform spectroscopy and spectroscopic ellipsometry at temperatures of 4–300 K. The normal-state reflectance of K \(_{0.8}\) Fe \(_{1.7}\) (Se \(_{0.73}\) S \(_{0.27}\) ) \(_2\) is analyzed using a Drude-Lorentz model with one Drude component. The temperature dependences of the plasma frequency, optical conductivity, scattering rate, and dc resistivity of the Drude contribution in the normal state are presented. In the superconducting state, we observe a signature of the superconducting gap opening at \(2\Delta (0)=11.8\)  meV. An abrupt decrease in the low-frequency dielectric permittivity \(\varepsilon _1(\omega )\) at \(T < T_c\) also evidences the formation of the superconducting condensate. The superconducting plasma frequency \(\omega _{pl,s} = (213\pm 5)\)  cm \(^{-1}\) and the magnetic penetration depth \(\lambda =(7.5\pm 0.2)\)   \(\mu\) m are determined.