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Anti-reduction of Ti4+ and improved quality factor in Cu-doped Ca0.61Nd0.26TiO3 ceramics

  • Dawei Gao,
  • Juncheng Ma,
  • Jiafen Zhang,
  • Qingang Shi,
  • Zhe Xiong,
  • Xing Zhang,
  • Bin Tang

摘要

The occurrence of "dark holes" is a common phenomenon in TiO2-based ceramics, resulting from the reduction of Ti4+ under high-temperature and low-oxygen partial pressure sintering conditions. To achieve low dielectric loss, Ca0.61Nd0.26Ti1-xCuxO3 ceramics were designed and prepared in this work. The results indicate that moderate doping of CuO not only enhances insulation resistivity and Q × f value but also reduces the positive τf value. The Ca0.61Nd0.26Ti0.98Cu0.02O3 sample exhibited the highest Q × f value of 16,895 GHz, contributing to the miniaturization and insertion loss of microwave devices.