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Synthesis of LiNi0.8Co0.1Mn0.1O2 cathode material with high energy density using di-butylamine as precipitant

  • Yan Wang,
  • Shishi Wei,
  • Chao Fan,
  • Geng Zhou,
  • Xiaocen Yan,
  • Yuanyuan Li,
  • Haowen Zhao,
  • Jiatai Wang,
  • Jian Li

摘要

The precursor synthesis of the LiNi0.8Co0.1Mn0.1O2 is usually adopted NaOH/NH3·H2O system. This method requires strict control of the pH value and feed rate. In this work, LiNi0.8Co0.1Mn0.1O2 was prepared by homogeneous precipitation method, and di-n-butylamine was used as the precipitant. The result shows that after calcination at 850 ℃ for 20 h, the initial discharge specific capacity of LiNi0.8Co0.1Mn0.1O2 cathode material is 210.66 mAh/g at a current density of 0.1 C. After 100 cycles, the specific discharge capacity is 192.29 mAh/g, and the capacity retention rate is 91.27%. This homogeneous precipitation method using di-n-butylamine as a precipitant allows the preparation of NCM-811 with excellent properties.