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Kill two birds with one stone: colorimetric/fluorescence immunosensor based on Au@Pt nanozyme for sensitive detection of imidacloprid

  • Rongqi Zhai,
  • Ge Chen,
  • Beibei Liu,
  • Guangyang Liu,
  • Xing Zhang,
  • Junjiang Liu,
  • Xiaomin Xu,
  • Yanguo Zhang,
  • Jing Wang,
  • Maojun Jin,
  • Donghui Xu

摘要

Gold-platinum (Au@Pt) nanozymes with high catalytic activity and stability were designed to improve the stability of the enzyme-linked immunosorbent assay (ELISA), and a two-mode signal output was used to enhance the sensitivity and confidence of the assay. This study reports the two-mode signal output based on Au@Pt nanozyme to catalyzed 3,3′,5,5′-tetramethylbenzidine (TMB) reaction. Oxidized 3,3′,5,5′-tetramethylbenzidine (ox-TMB) has wide absorption spectrum, providing excellent optical density capabilities and fluorescence quenching. The detection limits of imidacloprid were 0.88 μg/L and 1.14 μg/L in colorimetric and fluorescence modes, respectively. Multiple-mode strategy improves detection accuracy, increases the confidence of experimental results, and broadens detection modes. Two modes can meet the requirements of accurate and flexible multi-mode sensing in different application situations.

Graphical Abstract